Please use this identifier to cite or link to this item: https://hdl.handle.net/20.500.13091/4220
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dc.contributor.authorDolu, Taylan-
dc.contributor.authorNas, Bilgehan-
dc.date.accessioned2023-05-31T20:19:31Z-
dc.date.available2023-05-31T20:19:31Z-
dc.date.issued2023-
dc.identifier.issn0013-9351-
dc.identifier.issn1096-0953-
dc.identifier.urihttps://doi.org/10.1016/j.envres.2023.115731-
dc.identifier.urihttps://hdl.handle.net/20.500.13091/4220-
dc.description.abstractOne of the most consumed pharmaceutical subgroups across the world is nonsteroidal anti-inflammatory drugs (NSAIDs). However, the dissemination of these compounds to the natural environments through agronomic practices is a serious global problem. The hypothesis of this study is to reveal the transition of selected NSAIDs, paracetamol (PAR), diclofenac (DCF), ibuprofen (IBU), and naproxen (NAP) together with six main metabolites, detected in raw/treated wastewater (RWW/TWW) and sewage sludge generated in an urban wastewater treat-ment plant (WWTP) to soils and agricultural crops (corn, barley, sunflower, and sugar beet) through two widely applied agronomic practices, irrigation with TWW and application of sewage sludge as soil amendment. In other words, the cycles of 10 NSAIDs have been evaluated by simultaneously monitoring their concentrations in RWW/ TWW, sewage sludge, soils, and crops. It was determined that the parent compounds and detected metabolites were treated at quite higher removal efficiencies (93.4 - >99.9%) in the studied WWTP, while DCF was elim-inated poorly (7.9-52.2%). However, although it changes seasonally for some compounds, it was determined that the concentrations of almost all investigated NSAIDs increased at the determined irrigation points in the discharge channel (DC) where agricultural irrigations were performed. Apart from that, DCF, NAP, and 2-hydroxyibuprofen (2-OH-IBU) were always detected in sewage sludge seasonally up to about 20.5, 11.3, and 3.7 ng/g, respectively. While 2-OH-IBU was determined as the dominant metabolite in RWW, TWW, and sewage sludge, the metabolite of 1-hydroxyibuprofen (1-OH-IBU) was determined as the dominant compound in soils. Although 1-OH-IBU was not detected in TWW and sewage sludge in any season, detecting this metabolite as a common compound in all investigated soils (up to 60.1 ng/kg) reveals that this compound is the primary transformation product of IBU in soils. It was observed that at least one of the metabolites of IBU (1-OH-IBU and/ or 2-OH-IBU) was detected in all plants grown (up to 0.75 ng/g), especially during the periods when both agricultural practices were applied. In addition, the detection of 1-OH-IBU with increasing concentrations from root to shoots in corn grown as a result of both agronomic practices shows that this compound has a high translocation potential in the corn plant. Apart from this, it was determined that PAR was detected in corn (up to 43.3 ng/kg) and barley (up to 16.8 ng/kg) within the scope of irrigation with TWW, and NAP was detected in sugar beet (up to 11.2 ng/kg) through sewage sludge application.en_US
dc.description.sponsorshipKonya Technical University [202201053]; Konya Water and Sewerage Administration (KOSKI)en_US
dc.description.sponsorshipThis study was supported by Konya Technical University with a scientific research project number of 202201053. The authors also acknowledge the Konya Water and Sewerage Administration (KOSKI) for their support.en_US
dc.language.isoenen_US
dc.publisherAcademic Press Inc Elsevier Scienceen_US
dc.relation.ispartofEnvironmental Researchen_US
dc.rightsinfo:eu-repo/semantics/closedAccessen_US
dc.subjectAgricultural irrigationen_US
dc.subjectPharmaceuticalsen_US
dc.subjectPlant uptakeen_US
dc.subjectSewage sludgeen_US
dc.subjectSoil amendmenten_US
dc.subjectWastewater reuseen_US
dc.subjectPersonal Care Productsen_US
dc.subjectTransformation Productsen_US
dc.subjectEmerging Contaminantsen_US
dc.subjectDrinking-Wateren_US
dc.subjectPharmaceuticalsen_US
dc.subjectDegradationen_US
dc.subjectDiclofenacen_US
dc.subjectIbuprofenen_US
dc.subjectFateen_US
dc.subjectMicropollutantsen_US
dc.titleDissemination of nonsteroidal anti-inflammatory drugs (NSAIDs) and metabolites from wastewater treatment plant to soils and agricultural crops via real-scale different agronomic practicesen_US
dc.typeArticleen_US
dc.identifier.doi10.1016/j.envres.2023.115731-
dc.identifier.pmid36958380en_US
dc.identifier.scopus2-s2.0-85151292057en_US
dc.departmentKTÜNen_US
dc.authoridDOLU, Taylan/0000-0003-2331-1832-
dc.identifier.volume227en_US
dc.identifier.wosWOS:000966938900001en_US
dc.institutionauthor-
dc.relation.publicationcategoryMakale - Uluslararasi Hakemli Dergi - Kurum Ögretim Elemanien_US
dc.authorscopusid57214885046-
dc.authorscopusid12647682200-
dc.identifier.scopusqualityQ1-
item.fulltextWith Fulltext-
item.grantfulltextembargo_20300101-
item.cerifentitytypePublications-
item.languageiso639-1en-
item.openairetypeArticle-
item.openairecristypehttp://purl.org/coar/resource_type/c_18cf-
crisitem.author.dept02.06. Department of Environmental Engineering-
Appears in Collections:PubMed İndeksli Yayınlar Koleksiyonu / PubMed Indexed Publications Collections
Scopus İndeksli Yayınlar Koleksiyonu / Scopus Indexed Publications Collections
WoS İndeksli Yayınlar Koleksiyonu / WoS Indexed Publications Collections
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