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https://hdl.handle.net/20.500.13091/1324
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DC Field | Value | Language |
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dc.contributor.author | Steponaitis, Matas | - |
dc.contributor.author | La-Placa, Maria-Grazia | - |
dc.contributor.author | Kaya, İsmail Cihan | - |
dc.contributor.author | Bubniene, Giedre | - |
dc.contributor.author | Jankauskas, Vygintas | - |
dc.contributor.author | Daskeviciene, Maryte | - |
dc.contributor.author | Getautis, Vytautas | - |
dc.date.accessioned | 2021-12-13T10:38:44Z | - |
dc.date.available | 2021-12-13T10:38:44Z | - |
dc.date.issued | 2020 | - |
dc.identifier.issn | 2398-4902 | - |
dc.identifier.uri | https://doi.org/10.1039/d0se00728e | - |
dc.identifier.uri | https://hdl.handle.net/20.500.13091/1324 | - |
dc.description.abstract | In a short period of time, the rapid development of perovskite solar cells attracted a lot of attention in the science community with the record for power conversion efficiency being broken every year. Despite the fast progress in power conversion efficiency there are still many issues that need to be solved before starting large scale commercial applications, such as, among others, the difficult and costly synthesis and usage of toxic solvents for the deposition of hole transport materials (HTMs). We herein report new enamine-based charge transport materials obtainedviaa simple one step synthesis procedure, from commercially available precursors and without the use of expensive organometallic catalysts. The developed materials demonstrated rapid loss of mass during thermogravimetry analysis suggesting that they could be processed not only using solution processing but alsoviavacuum deposition. Furthermore, all HTMs demonstrated high charge carrier mobility withH2possessing the highest mobility of 2.5 x 10(-2)cm(2)V(-1)s(-1)under strong electric fields. The investigated materials were employed in vacuum-deposited p-i-n perovskite solar cells and champion devices with enamineH2demonstrate a PCE of 18.4%. | en_US |
dc.description.sponsorship | European Union's Horizon 2020 research and innovation program under PerTPV project [763977]; Research Council of LithuaniaResearch Council of Lithuania (LMTLT) [MIP-17-70]; Spanish Ministry of Science, Innovation and Universities [MAT2017-88821-R, RTI2018-095362-A-I00, EQC2018-004888-P]; Comunitat Valenciana [IDI-FEDER/2018/061]; TUBITAK 2214-A - International Doctoral Research Fellowship ProgrammeTurkiye Bilimsel ve Teknolojik Arastirma Kurumu (TUBITAK) | en_US |
dc.description.sponsorship | The research leading to these results had received funding from the European Union's Horizon 2020 research and innovation program under grant agreement No. 763977 of the PerTPV project. The authors acknowledge funding from the Research Council of Lithuania (grant No. MIP-17-70) and E. Kamarauskas for measurements of ionization potential. Further acknowledgments to the Spanish Ministry of Science, Innovation and Universities, MAT2017-88821-R, RTI2018-095362-A-I00 and EQC2018-004888-P, and the Comunitat Valenciana, IDI-FEDER/2018/061. I. C. K would like to thank TUBITAK 2214-A - International Doctoral Research Fellowship Programme for supporting his research at ICMol. M. S. acknowledges the Spanish Ministry for his RyC contract. | en_US |
dc.language.iso | en | en_US |
dc.publisher | ROYAL SOC CHEMISTRY | en_US |
dc.relation.ispartof | SUSTAINABLE ENERGY & FUELS | en_US |
dc.rights | info:eu-repo/semantics/openAccess | en_US |
dc.subject | P-I-N | en_US |
dc.subject | High-Performance | en_US |
dc.subject | Efficient | en_US |
dc.subject | Voltage | en_US |
dc.subject | Hysteresis | en_US |
dc.title | Enamine-based hole transporting materials for vacuum-deposited perovskite solar cells | en_US |
dc.type | Article | en_US |
dc.identifier.doi | 10.1039/d0se00728e | - |
dc.identifier.scopus | 2-s2.0-85092102820 | en_US |
dc.department | Fakülteler, Mühendislik ve Doğa Bilimleri Fakültesi, Metalurji ve Malzeme Mühendisliği Bölümü | en_US |
dc.authorid | Sessolo, Michele/0000-0002-9189-3005 | - |
dc.authorwosid | Sessolo, Michele/P-8911-2014 | - |
dc.authorwosid | Malinauskas, Tadas/J-7865-2012 | - |
dc.authorwosid | Bolink, Henk/L-7618-2014 | - |
dc.authorwosid | KAYA, Ismail Cihan/L-8046-2019 | - |
dc.identifier.volume | 4 | en_US |
dc.identifier.issue | 10 | en_US |
dc.identifier.startpage | 5017 | en_US |
dc.identifier.endpage | 5023 | en_US |
dc.identifier.wos | WOS:000573449300006 | en_US |
dc.relation.publicationcategory | Makale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanı | en_US |
dc.authorscopusid | 57191251478 | - |
dc.authorscopusid | 56553842600 | - |
dc.authorscopusid | 56966296500 | - |
dc.authorscopusid | 24337267700 | - |
dc.authorscopusid | 6602674489 | - |
dc.authorscopusid | 6506409327 | - |
dc.authorscopusid | 18134748900 | - |
dc.identifier.scopusquality | Q1 | - |
item.languageiso639-1 | en | - |
item.fulltext | With Fulltext | - |
item.cerifentitytype | Publications | - |
item.openairetype | Article | - |
item.grantfulltext | open | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
crisitem.author.dept | 02.11. Department of Metallurgical and Materials Engineering | - |
Appears in Collections: | Mühendislik ve Doğa Bilimleri Fakültesi Koleksiyonu Scopus İndeksli Yayınlar Koleksiyonu / Scopus Indexed Publications Collections WoS İndeksli Yayınlar Koleksiyonu / WoS Indexed Publications Collections |
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10.1039@D0SE00728E.pdf | 2.18 MB | Adobe PDF | View/Open |
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